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You may resign but if you do so without board approval, you will be in breach of your service agreement.
You may file your resignation at Companies House by filing form TM01: https://www.gov.uk/government/publications/terminate-an-appointment-of-a-director-tm01
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They may file legal proceedings against you for damages but they would need to show what loss they suffer as a result of you being in breach of contract.
If possible, you should notify the board that you wish to resign and seek their consent so that you are not in breach.
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